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Principals

 1887–1919   DR JOHN MARDEN

 BA LLD (Melbourne) 
 Principal of both Croydon and Pymble Colleges from 1916 
 1920–1929  DR E NEIL MCQUEEN
   MA (Melbourne) DSc (London) 
 Vice-Principal of both Colleges
 1929–1931  MISS ANNA DRENNAN
   Acting Principal MA (Edinburgh)
 Acting Principal at Pymble 1928
 1932-1941  MISS MARY HAMILTON
   BA DipEd (Melbourne) 
 1942-1945  DR HELEN ISABELLA WILKIE
   MA PhD (Edinburgh)
 Principal of PLC Armidale 1938 – 1941
 1946-1956  MISS EUNICE MACINDOE
   BSc (Sydney)
 1957  MISS JEAN TASSIE 
   Acting Principal, BA
 1958-1976  MISS FREDA L. WHITLAM
   BA DipEd (Melbourne) MA (Yale)
 1977  MRS NORMA BROWN
   Acting Principal, BA DipEd
 1978-1985   MISS PATRICIA DYSON
   MA DipEd (Sydney)
 1986-2010  DR WILLIAM MCKEITH AM
   BA DipEd (Macquarie) MA (Sydney) MBA (Leicester) EdD (Leicester), FACE FAIM 
 2011-present   DR PAUL BURGIS 
 

PhD (UNSW) MEd DipTeach DipDivMiss

Current Principal of Presbyterian Ladies' College, Sydney